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《International Journal of Hydrogen Energy》2022,47(81):34376-34386
Searching high-active, stable and abundant bifunctional catalysts to replace noble metals for hydrogen and oxygen evolution reactions (HER and OER) is desired. Herein, petal-like NiCoP sheets were synthesized on carbon paper covered with a 3D nitrogen-doped carbon nanofiber network (NiCoP/CNNCP) by a simple hydrothermal process followed by phosphorization. The HER overpotential in 0.5 M H2SO4 and OER overpotential in 1 M KOH of the NiCoP/CNNCP electrode only required 55 mV and 260 mV to drive a current density of 10 mA cm?2, respectively, which was comparable or even better than most nickel-and cobalt-based phosphide catalysts. The overall water-splitting electrolyzer with an asymmetric electrolyte system assembled using NiCoP/CNNCP as bifunctional electrodes required an extremely low cell voltage of 1.04 V to achieve a current density of 10 mA cm?2, which was much lower than almost all alkaline electrolysis systems. 相似文献
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《Ceramics International》2022,48(22):32973-32985
Multilayer structure design is one of the most promising methods for improving the comprehensive performance of AlCrN-based hard coatings applied to cutting tools. In this study, four types of AlCrSiN/AlCrVN/AlCrNbN multilayer coatings, with different modulated thicknesses, were deposited to investigate their microstructure, mechanical, tribological, and oxidizing properties. All multilayer coatings exhibited grain growth along the crystallographic plane of (200) with a NaCl-type face-centered cubic (FCC) structure. The results show that, as the modulation thickness decreases from ~35 nm to ~10 nm, (1) the grain refinement effect is increasingly evident; (2) all multilayer coatings show a hardness of >30 GPa and an elastic modulus of >300 GPa. Both the ability to resist elastic strain to failure and the plastic deformation of multilayer coatings increase. In addition, their resistance to cracking reduces; (3) the wear rates of these multilayer coatings reduce successively from 1.78 × 10?16 m3 N?1 m?1 to 7.7 × 10?17 m3 N?1 m?1. This is attributed to an increase in self-lubricating VOx and a decrease in adhesives from the counterparts; (4) the best high-temperature oxidation resistance was obtained for the multilayer coating with a modulated thickness of ~15 nm. 相似文献
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Shuang Chen Chao Yu Zhanfang Cao Xiaoping Huang Shuai Wang Hong Zhong 《International Journal of Hydrogen Energy》2021,46(10):7037-7046
The development of efficient and stable oxygen evolution reaction (OER) catalysts is an ongoing challenge. In order to solve the problem of low oxygen evolution efficiency of the current OER catalysts, a novel material was synthesized by the incorporation of NiFeCr-LDH and MoS2, and its structural and electrochemical properties were also investigated. The introduction of MoS2 improves the electrochemical performance of NiFeCr-LDH. The polarization curve shows that the potential of composite material is only 1.50 V at a current density of 10 mA cm?2, which is far superior to commercial precious metal catalysts. In addition, the stability experiment shows that the composite material has excellent stability, and the current density has little change after 500 cycles. Furthermore, we found that some metal ions, such as Ni, Cr and Mo, exist in the form of high valence on the surface of NiFeCr-LDH@MoS2, which is also conducive to the occurrence of oxygen evolution reaction. 相似文献
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Guiyong Zhang Zecong Chen Zhixiang Sui Dongsong Tao Zhicheng He Qian Tang Lei Sun 《International journal for numerical methods in engineering》2019,119(6):548-566
It is well known that the finite element method (FEM) encounters dispersion errors in coping with mid-frequency acoustic problems due to its “overly stiff” nature. By introducing the generalized gradient smoothing technique and the idea of condensed shape functions with virtual nodes, a cell-based smoothed radial point interpolation method is proposed to solve the Helmholtz equation for the purpose of reducing dispersion errors. With the properly selected virtual nodes, the proposed method can provide a close-to-exact stiffness of continuum, leading to a conspicuous decrease in dispersion errors and a significant improvement in accuracy. Numerical examples are examined using the present method by comparing with both the traditional FEM using four-node tetrahedral elements (FEM-T4) and the FEM model using eight-node hexahedral elements with modified integration rules (MIR-H8). The present cell-based smoothed radial point interpolation method has been demonstrated to possess a number of superiorities, including the automatically generated tetrahedral background mesh, high computational efficiency, and insensitivity to mesh distortion, which make the method a good potential for practical analysis of acoustic problems. 相似文献
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为提高稀疏表示跟踪模型性能,提出一种分段加权的反向稀疏跟踪算法,将跟踪问题转化为在贝叶斯框架下寻找概率最高的候选对象问题,构造不同的分段权重函数来分别度量候选目标与正负模板的判别特征系数。通过池化来降低跟踪结果的不确定性干扰,选择正负模板加权系数差值最大的候选表示作为跟踪结果。实验表明,在光照变化、遮挡、快速运动、运动模糊情况下,所提出的算法可以确保跟踪结果的准确性和鲁棒性。 相似文献
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《中国稀土学报(英文版)》2019,37(7):760-766
A novel process of calcification-leaching for bastnaesite concentrate(REFCO_3) was proposed. The prior calcification was carried out in the system of NaOH-CaO-H_2O and the lgC-pH pattern for Ce-F-Ca-C-H_2O system was drawn. The thermodynamics result indicates that decomposition for bastnaesite requires certain alkaline condition, but excessive alkalinity also causes decomposition of CaF_2. XRD and SEM-EDS analyses on the calcification-leaching process reveal that bastnaesite first decomposes into RE(OH)_3 and CaF_2. Then, by HCl leaching rare earths were extracted,while CaF_2 was left in the leaching residue. In addition, effects of temperature, time, NaOH and CaO on the calcification were investigated. The results show that the leaching rate of rare earths(REs)reaches 72.5 wt%, at the same time 99.2 wt% of F is left in leaching residue with 20 wt% NaOH and 38 wt% CaO at 493 K for 180 min. 相似文献
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目的 为了提高扫地机器人的自主性和智能化程度,为扫地机器人配备视觉传感器,使其获得视觉感知能力,通过研究有效的垃圾检测分类模型与算法,实现对垃圾的定位与识别,引导扫地机器人对垃圾进行自动识别与按类处理,提高工作的目的性和效率,避免盲动和减少能耗。方法 选择检测速度较快的YOLOv2作为主网络模型,结合密集连接卷积网络,嵌入深层密集模块,对YOLOv2进行改进,提出一种YOLOv2-dense网络,该网络可以充分利用图像的高分辨率特征,实现图像浅层和深层特征的复用与融合。结果 测试结果表明,智能扫地机器人使用本文方法可以有效识别不同形态的常见垃圾类别,在真实场景中,测试识别准确率为84.98%,目标检测速度达到26帧/s。结论 实验结果表明,本文构建的YOLOv2-dense网络模型具有实时检测的速度,并且在处理具有不同背景、光照、视角与分辨率的图片时,表现出较强的适应和识别性能。在机器人移动过程中,可以保证以较高的准确率识别出垃圾的种类,整体性能优于原YOLOv2模型。 相似文献
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